Div. of Synchrotron Radiation Research


E. Mårsell, C. L. Arnold, E. Lorek, D. Guenot, T. Fordell, M. Miranda, J. Mauritsson, H. Xu, A. LHuillier, and A. Mikkelsen
Secondary electron imaging of nanostructures using Extreme Ultra- Violet attosecond pulse trains and Infra-Red femtosecond pulses
Annalen der Physik, (2012) In Press

Surface electron dynamics unfold at time and length scales down to attoseconds and nanometres, making direct imaging with extreme spatiotemporal resolution highly desirable. However, this has turned out to be a major challenge even with the advent of reliable attosecond light sources. In this paper, we image photoelectrons from Ag nanowires and nanoparticles excited by extreme ultraviolet (XUV) attosecond pulse trains and infrared femtosecond pulses using a PhotoEmission Electron Microscope (PEEM). In addition, the samples were investigated using Scanning Electron Microscopy (SEM) and synchrotron based X-ray photoelectron spectroscopy (XPS). To achieve contrast between the nanostructures and the substrate in the XUV images, three different substrate materials were investigated: Cr, ITO and Au. We find that while plasmonic field enhancement can be observed on all three substrates, only on Au substrates do the Ag nanowires appear significantly brighter than the substrate in XUV-PEEM imaging. We perform 3-photon imaging of plasmonic hot-spots where the autocorrelation trace is observed in the interference signal between two femtosecond Infra-Red (IR) beams with sub-cycle precision. Finally, using Monte Carlo simulations, we show how the secondary electrons imaged in the XUV PEEM can potentially reveal information on the attosecond time scale from the near surface region of the nanostructures.

Link to the complete paper (if available):

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